Você não pode aumentar um RAID1 + 0 (não é suportado pelo mdadm).
De mdadm manpage:
Grow (or shrink) an array, or otherwise reshape it in some way. Currently supported growth options including changing the active size of component devices and changing the number of active devices in Linear and RAID levels 0/1/4/5/6, changing the RAID level between 0, 1, 5, and 6, and between 0 and 10, changing the chunk size and layout for RAID 0,4,5,6, as well as adding or removing a write-intent bitmap.