Claro que você pode. Eu uso iDump para essa finalidade. A iDump pode copiar todos os seus MP3s do seu iPod para o seu PC.
iDump will allow you transfer your songs off your iPod to a PC, iDump does come wrapped in installer but you can simply drop the .exe in the root directory on your iPod and run it from there.
Connect your iPod and run iDump and you'll have access to all your songs, select the songs you want to transfer then pick a destination directory and how you would like your songs to be named. And then sit back and transfer all the selected songs to the PC.
Aparentemente,oiDumpsófuncionaparaiPods,enãoparaiPhones.
Sevocêplanejausarosdois,
Change
Add and remove music, videos, playlists and artwork on your iPod.Backup
Backup all those tracks you just can't lose onto your computer. Import them automatically into your iTunes library.Share
SharePod can run straight from the iPod itself, so you can use it at work, school, home - wherever you and your iPod are.
iDump e SharePod são ambos gratuitos.